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Exciton Dynamics in Lead Halide Perovskite Nanocrystals: Recombination, Dephasing and Diffusion
Hardcover
Series: Springer Theses
Technology & EngineeringGeneral Science
ISBN13: 9783030709396
Publisher: Springer Nature
Published: May 19 2021
Pages: 152
Weight: 0.94
Height: 0.44 Width: 6.14 Depth: 9.21
Language: English
Less than a decade ago, lead halide perovskite semiconductors caused a sensation: Solar cells exhibiting astonishingly high levels of efficiency. Recently, it became possible to synthesize nanocrystals of this material as well. Interestingly; simply by controlling the size and shape of these crystals, new aspects of this material literally came to light. These nanocrystals have proven to be interesting candidates for light emission.
In this thesis, the recombination, dephasing and diffusion of excitons in perovskite nanocrystals is investigated using time-resolved spectroscopy. All these dynamic processes have a direct impact on the light-emitting device performance from a technology point of view. However, most importantly, the insights gained from the measurements allowed the author to modify the nanocrystals such that they emitted with an unprecedented quantum yield in the blue spectral range, resulting in the successful implementation of this material as theactive layer in an LED. This represents a technological breakthrough, because efficient perovskite light emitters in this wavelength range did not exist before.
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Exciton Dynamics in Lead Halide Perovskite Nanocrystals: Recombination, Dephasing and Diffusion
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