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  • Open Daily: 10am - 10pm
    Alley-side Pickup: 10am - 7pm

    3038 Hennepin Ave Minneapolis, MN
    612-822-4611

Open Daily: 10am - 10pm | Alley-side Pickup: 10am - 7pm
3038 Hennepin Ave Minneapolis, MN
612-822-4611
Design and Synthesis of N-Heterocyclic Donor Based Tadf Emitters for Application in Oleds

Design and Synthesis of N-Heterocyclic Donor Based Tadf Emitters for Application in Oleds

Zhang, Zhen

Paperback

Series: Beiträge Zur Organischen Synthese, Book 92

Chemistry

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ISBN10: 3832551670
ISBN13: 9783832551674
Publisher: Logos Verlag Berlin
Published: Sep 15 2020
Pages: 249
Weight: 0.75
Height: 0.56 Width: 5.68 Depth: 8.04
Language: English
As one of the most promising electroluminescent technologies, thermally activated delayed fluorescence (TADF) OLEDs have attracted more and more attention due to their enormous and unique potential for application in industrial products. The presented work is focused on the development of new TADF emitters for OLEDs. Particularly, emitters for blue TADF emission are thoroughly investigated via the evaluation of newly designed and modified N-heterocyclic donors. In the first part, TADF emitters based on N-heterocyclic donors and boron-containing acceptors were designed and synthesized. Photophysical studies revealed that blue emission was accessed through the variation of the N-heterocyclic donors. Secondly, a series of TADF emitters derived from the indolocarbazole donors and di-phenyltriazine acceptors were evaluated. OLED with the EQE of over 22.1 % and sky-blue emission at 483 nm was obtained. Lastly, deep blue TADF emission was realized by introducing electron-withdrawing groups to the [2.2]paracyclophane-derived donor unit. For further decreasing the DeltaE_{STto harvest more efficient TADF molecules, through-space donor dimers and the corresponding emitters were also synthesized, yielding blue TADF emission.

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