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Catalytic and Process Study of the Selective Hydrogenation of Acetylene and 1,3-Butadiene
Hardcover
Series: Springer Theses
ISBN13: 9789811007729
Publisher: Springer Nature
Published: Jan 12 2017
Pages: 141
Weight: 0.88
Height: 0.44 Width: 6.14 Depth: 9.21
Language: English
This thesis offers novel methods for catalyst and process design for the selective hydrogenation of acetylene and 1,3-butadiene. The author predicts the properties of supported Pd-Ni bimetallic catalysts using density functional theory (DFT) calculations and temperature-programmed desorption (TPD). The excellent correlation between model surfaces and supported catalysts demonstrates the feasibility of designing effective bimetallic catalysts for selective hydrogenation reactions. The author also proposes a method for designing non-precious metal catalysts to replace precious metals. She modifies the process of selective hydrogenation of acetylene by coupling the selective adsorption to the selective hydrogenation in the liquid phase, as a result of which the ethylene selectivity is greatly improved and heat transfer is greatly enhanced. Lastly, by analyzing the mechanism of liquid-phase hydrogenation, the author proposes a multi-stage slurry bed reactor for industrial applications.
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